Quantum Nonlinear Optics with Polar J-Aggregates in Microcavities.

نویسندگان

  • Felipe Herrera
  • Borja Peropadre
  • Leonardo A Pachon
  • Semion K Saikin
  • Alán Aspuru-Guzik
چکیده

We predict that an ensemble of organic dye molecules with permanent electric dipole moments embedded in a microcavity can lead to strong optical nonlinearities at the single-photon level. The strong long-range electrostatic interaction between chromophores due to their permanent dipoles introduces the desired nonlinearity of the light-matter coupling in the microcavity. We develop a semiclassical model to obtain the absorption spectra of a weak probe field under the influence of strong exciton-photon coupling with the cavity field. Using realistic parameters, we demonstrate that a cavity field with an average photon number near unity can significantly modify the absorptive and dispersive response of the medium to a weak probe field at a different frequency. Finally, we show that the system is in the regime of cavity-induced transparency with a broad transparency window for dye dimers. We illustrate our findings using pseudoisocyanine chloride (PIC) J-aggregates in currently available optical microcavities.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Strong exciton-photon coupling in inorganic-organic multiple quantum wells embedded low-Q microcavity.

Optoelectronic-compatible heterostructures are fabricated from layered inorganic-organic multiple quantum wells (IO-MQW) of Cyclohexenyl ethyl ammonium lead iodide, (C(6)H(9)C(2)H(4)NH(3))(2)PbI(4) (CHPI). These hybrids possess strongly-resonant optical features, are thermally stable and compatible with hybrid photonics assembly. Room-temperature strong-coupling is observed when these hybrids a...

متن کامل

Semiconductor Optical Microcavities for Chip-Based Cavity QED

Optical microcavities can be characterized by two key quantities: an effective mode volume Veff, which describes the per photon electric field strength within the cavity, and a quality factor Q, which describes the photon lifetime within the cavity. Cavities with a small Veff and a high Q offer the promise for applications in nonlinear optics, sensing, and cavity quantum electrodynamics (cavity...

متن کامل

Tunable resonant optical microcavities by self-assembled templating.

Micrometer-scale optical cavities are produced by a combination of template sphere self-assembly and electrochemical growth. Transmission measurements of the tunable microcavities show sharp resonant modes with Q factors of >300 and 25-fold local enhancement of light intensity. The presence of transverse optical modes confirms the lateral confinement of photons. Calculations show that submicrom...

متن کامل

Many-body physics of a quantum fluid of exciton-polaritons in a semiconductor microcavity

Some recent results concerning nonlinear optics in semiconductor microcavities are reviewed from the point of view of the many-body physics of an interacting photon gas. Analogies with systems of cold atoms at thermal equilibrium are drawn, and the peculiar behaviours due to the non-equilibrium regime pointed out. The richness of the predicted behaviours shows the potentialities of optical syst...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • The journal of physical chemistry letters

دوره 5 21  شماره 

صفحات  -

تاریخ انتشار 2014